• Carbon Fiber-Carbon Black Synergistically Reinforced Liquid Silicone Rubber Composite for Stretchable Conductive Materials

  • Xiaoyong Hao†

  • Hebei Huabei Petroleum RONGSHENG Machinery Manufacturing Co., Ltd., Renqiu, Hebei 062550, China

  • 탄소섬유-카본블랙 상승 전도 네트워크 기반 신축성 전도성 액상 실리콘 고무 복합재료

  • Reproduction, stored in a retrieval system, or transmitted in any form of any part of this publication is permitted only by written permission from the Polymer Society of Korea.

References
  • 1. Yang, Y.; Deng, H.; Fu, Q. Recent Progress on PEDOT:PSS Based Polymer Blends and Composites for Flexible Electronics and Thermoelectric Devices. Mater. Chem. Front. 2020, 4, 3130-3152.
  •  
  • 2. Zhang, F.-T.; Xu, L.; Chen, J.-H.; Zhao, B.; Fu, X.-Z.; Sun, R.; Chen, Q.; Wong, C.-P. Electroless Deposition Metals on Poly(dimethylsiloxane) with Strong Adhesion As Flexible and Stretchable Conductive Materials. ACS Appl. Mater. Interfaces 2018, 10, 2075-2082.
  •  
  • 3. Amjadi, M.; Turan, M.; Clementson, C. P.; Sitti, M. Parallel Microcracks-based Ultrasensitive and Highly Stretchable Strain Sensors. ACS Appl. Mater. Interfaces 2016, 8, 5618-5626.
  •  
  • 4. Tee, B. C. K.; Ouyang, J. Y. Soft Electronically Functional Polymeric Composite Materials for a Flexible and Stretchable Digital Future. Adv. Mater. 2018, 30, 1802560.
  •  
  • 5. Xu, D.; Wang, Q.; Feng, D.; Liu, P. Facile Fabrication of Multifunctional Poly(ethylene-co-octene)/Carbon Nanotube Foams Based on Tunable Conductive Network. Ind. Eng. Chem. Res. 2020, 59, 1934-1943.
  •  
  • 6. Markov, A.; Wördenweber, R.; Ichkitidze, L.; Gerasimenko, A.; Kurilova, U.; Suetina, I.; Mezentseva, M.; Offenhäusser, A.; Telyshev, D. Biocompatible SWCNT Conductive Composites for Biomedical Applications, Nanomaterials, 2020, 10, 2492.
  •  
  • 7. Chang, M.; Li, Y.; Xu, L.; Wang, W.; Wang, C.; Wang, R. A Novel Assembled Carbon Black/carbon Nanotubes (CB/MWCNT) Nano-structured Composite for Pressure-sensitive Conductive Silicon Rubber (SR). J. Mater. Sci.: Mater. Electron. 2018,29, 2716-2724.
  •  
  • 8. Chen, Y.-F.; Huang, M.-L.; Cai, J.-H.; Weng, Y.-X.; Wang, M. Piezoresistive Anisotropy in Conductive Silicon Rubber/multi-walled Carbon Nanotube/nickel Particle Composites via Alignment of Nickel Particles. Compos. Sci. Technol. 2022, 225, 109520.
  •  
  • 9. Lu, Y.; Wang, J.; Wang, L.; Zhao, D.; Song, S. Construction of 3D Carbon Fiber/carbon Nanotube/silicone Rubber Nanocomposites for Stretchable Conductors Through Interface Host-guest Dendrimers. Compos. Sci. Technol. 2021, 205, 108692.
  •  
  • 10. Lin, Y.; Liu, S.; Peng, J.; Liu, L. Constructing a Segregated Graphene Network in Rubber Composites Towards Improved Electrically Conductive and Barrier Properties. Compos. Sci. Technol. 2016, 131, 40-47.
  •  
  • 11. Song, P.; Wang, G.; Zhang, Y. Preparation and Performance of Graphene/carbon Black Silicone Rubber Composites Used for Highly Sensitive and Flexible Strain Sensors. Sens. Actuators, A. 2021, 323, 112659.
  •  
  • 12. Yang, Z.; Liu, H.; Wu, S.; Tang, Z.; Guo, B.; Zhang, L. A Green Method for Preparing Conductive Elastomer Composites With Interconnected Graphene Network via Pickering Emulsion Templating. Chem. Eng. J. 2018, 342, 112-119.
  •  
  • 13. Luo, S. D.; Liu, T. SWCNT/Graphite Nanoplatelet Hybrid Thin Films for Self-Temperature- Compensated, Highly Sensitive, and Extensible Piezoresistive Sensors. Adv. Mater. 2013, 25, 5650-5657.
  •  
  • 14. Segev-Bar, M.; Haick, H. Flexible Sensors Based on Nanoparticles. ACS Nano 2013, 7, 8366-8378.
  •  
  • 15. Tang, M.; Jiang, Z.; Wang, Z.; Qin, Y.; Jiang, Y.; Wu, L.; Li, Z. High-adhesion PDMS/Ag Conductive Composites for Flexible Hybrid Integration. Chem. Eng. J. 2023, 451, 138730.
  •  
  • 16. Zhang, H.; Liu, N.; Shi, Y.; Liu, W.; Yue, Y.; Wang, S.; Ma, Y.; Wen, L.; Li, L.; Long, F.; Zou, Z.; Gao, Y. Piezoresistive Sensor with High Elasticity Based on 3D Hybrid Network of Sponge@CNTs @Ag NPs. ACS Appl. Mater. Interfaces 2016, 8, 22374-22381.
  •  
  • 17. Huang, P.; Xia, Z.; Cui, S. 3D Printing of Carbon Fiber-filled Conductive Silicon Rubber. Mater. Des. 2018, 142, 11-21.
  •  
  • 18. Azizkhani, M. B.; Kadkhodapour, J.; Rastgordani, S.; Anaraki, A. P.; Shirkavand Hadavand, B. Highly Sensitive, Stretchable Chopped Carbon Fiber/Silicon Rubber Based Sensors for Human Joint Motion Detection. Fibers Polym. 2019, 20, 35-44.
  •  
  • 19. Yang, H.; Gong, L. H.; Zheng, Z.; Yao, X. F. Highly Stretchable and Sensitive Conductive Rubber Composites with Tunable Piezoresistivity for Motion Detection and Flexible Electrodes. Carbon 2020,158, 893-903.
  •  
  • 20. Huang, P.; Xia, Z.; Cui, S.; Wang, J.; Zhao, S. Potential Temperature Sensing of Oriented Carbon-fiber Filled Composite and Its Resistance Memory Effect. J. Mater. Sci.: Mater. Electron. 2019, 30, 9612-9622.
  •  
  • 21. Li, Y.; Liu, G.; Wang, L.; Zhang, J.; Xu, M.; Shi, S. Q. Multifunctional Conductive Graphite/cellulosic Microfiber-natural Rubber Composite Sponge with Ultrasensitive Collision-warning and Fire-warning. Chem. Eng. J. 2022, 431, 134046.
  •  
  • Polymer(Korea) 폴리머
  • Frequency : Bimonthly(odd)
    ISSN 2234-8077(Online)
    Abbr. Polym. Korea
  • 2025 Impact Factor : 1.0
  • Indexed in SCIE

This Article

  • 2026; 50(4): 544-553

    Published online Jul 25, 2026

  • 10.7317/pk.2026.50.4.544
  • Received on Feb 25, 2026
  • Revised on Apr 16, 2026
  • Accepted on Apr 28, 2026

Correspondence to

  • Xiaoyong Hao

  • Hebei Huabei Petroleum RONGSHENG Machinery Manufacturing Co., Ltd., Renqiu, Hebei 062550, China

  • E-mail: 772914312@qq.com